Upsampling is basically padding zeros in between signal samples and then interpolation. The interpolation itself is a low pass filter. The rcosdesign is a low pass filter so after zero padding by factor of 3, you need to convolve the resulting zero padded sequence with this filter.
Note that: it is not an ideal filter, so you would get varied attenuation for different frequencies for the discrete time frequency repsonse after convolving with this filter.
Further, remember you would be "drawing in" frequency components from other periodic repetitions of the discrete time frequency response of the original sequence immediately after zero padding, these would appear in the high frequencies of your $-\pi$ to $\pi$ spectrum hence roll off and spectrum of original sequence would decide the amount of alisaing and distortion of the original signal's frequency response.
As an example if your original sequence is bandlimited in $-\pi/4$ to $\pi/4$. Then this would shrink to $-\pi/12$ to $\pi/12$ after upsampling by 3 but you would also get frequency components to the left of $-7\pi/12$ and right of $7\pi/12$. So in this example make sure your roll of begins at $-\pi/12$ and $\pi/12$ and frequency resonse of filter decays very much to 0 before $7\pi/12$ and $-7\pi/12$
Sample MATLAB code below:
Sampling period implied and ignore the time scale:
close all;
clear all;
clc;
t=-5:0.1:5;
T=5;
RECT=rectpuls(t,T);
FFT_size=1024;
signal_fft=fft(RECT,FFT_size);
signal_up=upsample(RECT,3);
signalup_fft=fft(signalup,FFT_size);
h=rcosdesign(0.25,64,2);
H=fft(h,FFT_size);
Product=H.*signalup_fft;
filtered_sequence=ifft(Product,FFT_size);
figure;
subplot(6,1,1);
plot(t,RECT);
ylim([-2 2]);
xlim([-5 5]);
title('original signal');
subplot(6,1,2);
plot(fftshift(abs(signal_fft)));
title('frequency response of original signal,periodicity implied');
subplot(6,1,2);
plot(fftshift(abs(signal_fft)));
title('frequency response of original signal,periodicity implied');
subplot(6,1,3);
plot(fftshift(abs(signalup_fft)));
title('frequency response of upsampled signal,periodicity implied');
subplot(6,1,4);
plot(fftshift(abs(H)));
title('frequency response of rcosdesign filter,periodicity implied');
subplot(6,1,5);
plot(fftshift(abs(Product)));
title('frequency response of filtered sequence,periodicity implied');
subplot(6,1,5);
plot(filtered sequence);
title('recovered signal, ignore time scale');
